New UV-LED frontal flow photocatalytic reactor for VOCs treatment: Compactness, intensification and optimization studies

نویسندگان

چکیده

This study investigates and provides a solution for optimizing the photocatalytic treatment of toxic gases based on use TiO2 media deposited luminous textiles. The target was cyclohexane referent type A gas filtration tests. supports were characterized by scanning electron microscopy. Then, experiments conducted batch reactor showed that TiO2-coated optical fiber (in situ illumination configuration) performs better than conventional configuration (cellulosic with external radiation ''UV lamp''. To take advantage new configuration, an intensification carried out increasing amount in UV intensities LED. Increasing these two parameters leads to approximately fourfold increase degradation rate. continuous allowed highlight efficiency front flow reactors developed (PFR-LED) compared configuration. increased is demonstrated specific rate optimized PFR-LED reactor. performance evaluation compact configurations frontal (PFR-LED Optimized) aimed influence inlet concentration under different rates. Furthermore, effect number shows selectivity are enhanced. results obtained using four (4OF/4UV-LED) 1.19 mmol·m−3 input at 18 L.min−1 optimal humidity conditions (38 %), constituting ultimate CO2 achieved (31 %) abatement 59 %. global investigation has design version economical efficient way eliminate gaseous pollutants, which clearly meets main aims UN Sustainable Development Goals (UN SDGs).

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ژورنال

عنوان ژورنال: Chemical Engineering Journal

سال: 2023

ISSN: ['1873-3212', '1385-8947']

DOI: https://doi.org/10.1016/j.cej.2022.138784